Integrated Surface-to-Bulk Engineering of Li-Rich Mn-Based Cathodes for Reversible Oxygen Redox and Enhanced Interfacial Stability Under Broad-Temperature Conditions.
The pursuit of high-energy-density lithium-ion batteries has established lithium-rich manganese-based layered oxides (LRMs) as compelling cathode candidates. However, their practical application is hindered by irreversible oxygen loss, interfacial degradation, and sluggish reaction kinetics. Notably, kinetic limitation...