Mechanically, Thermally, and Interfacially Robust Solid Polymer Electrolytes Enabled by an Organic-Inorganic Interwoven Architecture.
Solid polymer electrolytes (SPEs) are promising for use in high-energy-density solid-state Li metal batteries. However, their practical application is hindered by challenges including poor mechanical strength, inadequate thermal stability, electrode-interface instability, and sluggish ionic transport, which collectivel...