A Fully Frequency-Dependent Formulation of the Open Quantum System Polarizable Continuum Model
We introduce a fully frequency-dependent formulation of the open quantum system polarizable continuum model (OQS-PCM), as derived from the non-Markovian time-dependent stochastic Schrödinger equation for a polarizable bath in the limit of averaging out the stochastic fluctuations. OQS-PCM(ω) captures the delayed coupli...