Elucidating how the surface structure alters reaction networks during cycloalkane dehydrogenation remains critical for understanding and mitigating catalyst deactivation. Here, we show that early deactivation of Pt catalysts in cycloalkane dehydrogenation is linked to structure-sensitive pathway branching of a partia...
S. Han, Kiheon Sung, ByeongJo Shim et al.· JACS Au· 0 citations
Electrochemical CO
2
conversion in acid can, in principle, maximize carbon efficiency but is typically undermined by facile hydrogen evolution. Moreover, operating at high current density often triggers a sharp local pH increase that propagates into the bulk electrolyte, causing an overall pH shift that erodes no...
Jeonguk Hwang, Yoonjun Cho, Yoojin Lee et al.· Advanced Energy Materials· 0 citations
High‐temperature CO
2
electrolysis is a promising route for sustainable fuel production and carbon utilization, yet its efficiency is limited by the scarcity of highly active electrode materials. This study demonstrates heterointerface engineering as a key strategy to dramatically enhance the performance of the c...