Interlayer Metal‐Ligand Coordination in Covalent Organic Frameworks: A Structural Strategy for Enhanced Nitrate Reduction Electrocatalysis
Efficient multielectron electrocatalysis in layered covalent organic frameworks (COFs) is frequently limited by weak cross‐plane charge delivery to pore‐confined active sites. Herein, we report the construction of two metal‐bridged COFs (Py1‐COF‐Cu and Py2‐COF‐Cu) by incorporating nitrogen‐containing heterocycles to fa...