On the Electronic Path-Integral Normal Modes of the Spin-Mapping Representation of Nonadiabatic Dynamics
Nonadiabatic Matsubara dynamics has been proposed in both the Meyer-Miller-Stock-Thoss (MMST) and spin-mapping representations, whereby the dynamics are truncated in the higher path-integral normal modes of the nuclear degrees of freedom, but no truncation is performed in the electronic variables. In contrast to single...