Deciphering Dynamic Self-Healing for Crystallinity Control in β-Ketoenamine-Linked Covalent Organic Frameworks.
Covalent organic frameworks derived from triformylphloroglucinol (Tp-COFs) represent a prominent branch of COFs due to their high potential in separation, energy storage, and optoelectronics. However, the development of Tp-COFs is often hindered by limited crystallinity, resulting from the low reversibility of β-ketoen...