Topology-Directed Biomimetic Confinement in Covalent Organic Frameworks Couples Electrocatalytic Water Activation to Reactive Oxygen Species Evolution for Dual-Potential Electrochemiluminescence.
Enzymatic confined microenvironments cooperatively modulate reactive oxygen species (ROS) dynamics to enhance biocatalytic efficiency. Drawing inspiration from this natural mechanism, we developed covalent organic frameworks (COFs) with programmable nanoscale confinement, achieved via topology-directed assembly. This d...