Tautomeric-State Engineering of Anthraquinone Covalent Organic Frameworks Enables Efficient H2O2 Photosynthesis from Water and Oxygen.
Hydrogen peroxide photosynthesis from water and oxygen represents a sustainable route toward decentralized chemical manufacturing, yet its efficiency is severely restricted by sluggish water oxidation reaction. Herein, we report an alkaline-triggered keto-form reconstruction strategy in an anthraquinone-based covalent...