Electronic Isolation Wall Engineering in Covalent Organic Frameworks for Enhancing Overall H2O2 Photosynthesis
Covalent organic frameworks (COFs) hold promises for overall H2O2 photosynthesis. However, their efficiency is constrained by rapid charge recombination at the universal C=N linkages due to the nitrogen lone pairs acting as efficient hole traps. Here, we report a molecular-level electronic isolation strategy through...