The sluggish kinetics of the water oxidation reaction (WOR) remain the primary bottleneck for photocatalytic H2O2 production. Beyond traditional band-structure engineering, modulating the pore microenvironment to synchronize mass transfer and charge kinetics is crucial yet challenging. Here, we report a channel-wall en...
The escalating depletion of fossil fuels, rising greenhouse gas emissions, and pervasive plastic pollution pose unprecedented threats to the environment and human well-being, underscoring an urgent need for sustainable and clean resource recycling technologies. Solar-driven photoreforming of plastic waste simultaneousl...
Hai-Yin Zhan, Guan-Qi Yu, Xiang-Kun Jia et al.· Advances in Materials· 0 citations
Precise oxidant activation is essential for advanced water treatment but is often limited by radical quenching and low oxidant efficiency. Peroxymonosulfate (PMS) is promising; however, directing O-O cleavage towards non-radical pathways requires tightly coupled proton‒electron transfer, which is rarely achieved in het...