Facet Modulation of Interfacial Water Structure Tunes Electrocatalytic Hydrogen Reaction Kinetics
Interfacial water structure is theoretically envisioned as the master regulator of electrocatalytic reaction kinetics, but the direct experimental validation of this role has remained a formidable challenge. Probing kinetic isotope effects (KIEs) is paramount to deciphering the elusive proton-coupled electron transfe...