Molecularly Engineered Self-Assembled Molecular Layer for pH-Tolerant CO2 Electroreduction With Enhanced Activity and Stability.
The electrochemical CO2 reduction is crucial for achieving carbon neutrality, wherein the catalytic performance is governed not only by the intrinsic catalytic activity but also by the microenvironment of the triple-phase interface. In this study, a self-assembled molecular (SAM) of trimethoxy(3,3,3-trifluoropropyl)sil...