Programming High‐Density Mesoporosity in Monodispersed MOF Single Crystals via Inherent Jahn–Teller Distortion
Incorporating high‐density mesoporosity into single crystals has long posed a fundamental challenge, as traditional pore‐engineering methods inevitably impair long‐range crystalline order. Here, we repurpose an inherent crystallographic defect—the Jahn–Teller distortion (JTD)—as a programmable tool for encoding mesopor...