Oxidation State of Sulfur Modification Controls the CO2 Electroreduction Activity of Fe(III) Porphyrin Catalysts
Yu-Zhe Jian
Ben-Xing Mei
Ling-Rui Shi
Yu-Han Xu
An-Hao Han
Jin-Kun Liu
Jing Guan
Cheng-Yu Liu
Rui Cao
Abstract
Secondary-sphere sulfur doping can effectively modulate the electrocatalytic CO2 reduction reaction (CO2RR) performance of single-atom catalysts (SACs). However, the precise modulation mechanism of sulfur species remains poorly understood due to...